Recycling of lithium-ion batteries: a brief review of processes, advancements, and prospects
DOI:
https://doi.org/10.47456/bjpe.v10i1.42817Keywords:
Biometallurgy, Waste Management, Hydrometallurgy, Thermal induction, PyrometallurgyAbstract
This work presents a brief review of conventional (pyrometallurgy and hydrometallurgy) and alternative recycling processes of LIBs (direct recycling, bio-metallurgy, electric field, and thermal induction), which are responsible for recovering valuable materials such as Li, Ni, Co, Mn, Cu, Al and graphite. Bibliographic and documental research was used to state comparisons between different technologies. Research findings reveal that alternative recycling is more efficient and sustainable when compared to conventional methods. However, the commercial use of conventional processes persists due to their established technologies and large-scale production infrastructure. Therefore, overcoming technological bottlenecks associated with alternative recycling will support the lithium battery (LIB) production chain, meeting the growing demand in the electric vehicle market. Technological challenges need to foster the development of innovative and sustainable recycling technologies for lithium batteries in line with solid waste management policies.
Downloads
References
Bhar, M., Bhattacharjee, U., Yalamanchili, K., & Martha, S. K. (2023). Effective upcycling of waste separator and boosting the electrochemical performance of recycled graphite anode for lithium-ion batteries. Journal of Power Sources, 580, 233403. https://doi.org/10.1016/J.JPOWSOUR.2023.233403 DOI: https://doi.org/10.1016/j.jpowsour.2023.233403
Dong, C., Dong, X., Jiang, Q., Dong, K., & Liu, G. (2018). What is the probability of achieving the carbon dioxide emission targets of the Paris Agreement? Evidence from the top ten emitters. Science of The Total Environment, 622-623, 1294-1303. https://doi.org/10.1016/J.SCITOTENV.2017.12.093 DOI: https://doi.org/10.1016/j.scitotenv.2017.12.093
Du, K., Ang, E. H., Wu, X., & Liu, Y. (2022). Progresses in Sustainable Recycling Technology of Spent Lithium-Ion Batteries. Energy & Environmental Materials, 5(4), 1012-1036. https://doi.org/10.1002/EEM2.12271 DOI: https://doi.org/10.1002/eem2.12271
Feng, C. C., Chang, K. F., Lin, J. X., Lee, T. C., & Lin, S. M. (2022). Toward green transition in the post Paris Agreement era: The case of Taiwan. Energy Policy, 165, 112996. https://doi.org/10.1016/J.ENPOL.2022.112996 DOI: https://doi.org/10.1016/j.enpol.2022.112996
Golmohammadzadeh, R., Faraji, F., & Rashchi, F. (2018). Recovery of lithium and cobalt from spent lithium ion batteries (LIBs) using organic acids as leaching reagents: A review. Resources, Conservation and Recycling, 136, 418-435. https://doi.org/10.1016/J.RESCONREC.2018.04.024 DOI: https://doi.org/10.1016/j.resconrec.2018.04.024
Goodenough, J. B., & Park, K. S. (2013). The Li-ion rechargeable battery: A perspective. Journal of the American Chemical Society, 135(4), 1167-1176. https://doi.org/10.1021/JA3091438/ASSET/IMAGES/MEDIUM/JA-2012-091438_0009.GIF DOI: https://doi.org/10.1021/ja3091438
Horeh, N. B., Mousavi, S. M., & Shojaosadati, S. A. (2016). Bioleaching of valuable metals from spent lithium-ion mobile phone batteries using Aspergillus niger. Journal of Power Sources, 320, 257-266. https://doi.org/10.1016/J.JPOWSOUR.2016.04.104 DOI: https://doi.org/10.1016/j.jpowsour.2016.04.104
IEA. (2023). Electric Vehicles.
Jin, S., Mu, D., Lu, Z., Li, R., Liu, Z., Wang, Y., Tian, S., & Dai, C. (2022). A comprehensive review on the recycling of spent lithium-ion batteries: Urgent status and technology advances. Journal of Cleaner Production, 340, 130535. https://doi.org/10.1016/J.JCLEPRO.2022.130535 DOI: https://doi.org/10.1016/j.jclepro.2022.130535
Kader, Z. A., Marshall, A., & Kennedy, J. (2021). A review on sustainable recycling technologies for lithium-ion batteries. Emergent Materials, 4(3), 72-735. https://doi.org/10.1007/S42247-021-00201-W/FIGURES/4 DOI: https://doi.org/10.1007/s42247-021-00201-w
Kasprzak, W., Li, D., Patience, G. S., Sauriol, P., Amaris, H. V., Dolle, M., Gauthier, M., Rousselot, S., Talebi-Esfandarani, M., Bibienne, T., Sun, X., Liu, Y., & Liang, G. (2017). Using induction melting to make lithium-ion battery material. Advanced Materials & Processes, 175(8), 16-23. DOI: https://doi.org/10.31399/asm.amp.2017-08.p016
Khabbazan, M. M., & von Hirschhausen, C. (2021). The implication of the Paris targets for the Middle East through different cooperation options. Energy Economics, 104, 105629. https://doi.org/10.1016/J.ENECO.2021.105629 DOI: https://doi.org/10.1016/j.eneco.2021.105629
Kim, S., Bang, J., Yoo, J., Shin, Y., Bae, J., Jeong, J., Kim, K., Dong, P., & Kwon, K. (2021). A comprehensive review on the pretreatment process in lithium-ion battery recycling. Journal of Cleaner Production, 294, 126329. https://doi.org/10.1016/J.JCLEPRO.2021.126329 DOI: https://doi.org/10.1016/j.jclepro.2021.126329
Kriston, A., Kersys, A., Antonelli, A., Ripplinger, S., Holmstrom, S., Trischler, S., Döring, H., & Pfrang, A. (2020). Initiation of thermal runaway in Lithium-ion cells by inductive heating. Journal of Power Sources, 454, 227914. https://doi.org/10.1016/J.JPOWSOUR.2020.227914 DOI: https://doi.org/10.1016/j.jpowsour.2020.227914
Lai, X., Chen, Q., Tang, X., Zhou, Y., Gao, F., Guo, Y., Bhagat, R., & Zheng, Y. (2022). Critical review of life cycle assessment of lithium-ion batteries for electric vehicles: A lifespan perspective. ETransportation, 12, 100169. https://doi.org/10.1016/J.ETRAN.2022.100169 DOI: https://doi.org/10.1016/j.etran.2022.100169
Leal, V. M., Ribeiro, J. S., Coelho, E. L. D., & Freitas, M. B. J. G. (2023). Recycling of spent lithium-ion batteries as a sustainable solution to obtain raw materials for different applications. Journal of Energy Chemistry, 79, 118-134. https://doi.org/10.1016/J.JECHEM.2022.08.005 DOI: https://doi.org/10.1016/j.jechem.2022.08.005
Li, J., Li, L., Yang, R., & Jiao, J. (2023). Assessment of the lifecycle carbon emission and energy consumption of lithium-ion power batteries recycling: A systematic review and meta-analysis. Journal of Energy Storage, 65, 107306. https://doi.org/10.1016/J.EST.2023.107306 DOI: https://doi.org/10.1016/j.est.2023.107306
Li, L., Zhang, X., Li, M., Chen, R., Wu, F., Amine, K., & Lu, J. (2018). The Recycling of Spent Lithium-Ion Batteries: a Review of Current Processes and Technologies. Electrochemical Energy Reviews 2018 1(4), 461-482. https://doi.org/10.1007/S41918-018-0012-1 DOI: https://doi.org/10.1007/s41918-018-0012-1
Li, P., Luo, S., Zhang, L., Liu, Q., Wang, Y., Lin, Y., Xu, C., Guo, J., Cheali, P., & Xia, X. (2023). Progress, challenges, and prospects of spent lithium-ion batteries recycling: A review. Journal of Energy Chemistry. https://doi.org/10.1016/J.JECHEM.2023.10.012 DOI: https://doi.org/10.1016/j.jechem.2023.10.012
Liao, X., Ye, M., Liang, J., Jian, J., Li, S., Gan, Q., Liu, Z., Mo, Z., Huang, Y., & Sun, S. (2023). Comprehensive insights into the gallic acid assisted bioleaching process for spent LIBs: Relationships among bacterial functional genes, Co(III) reduction and metal dissolution behavior. Journal of Hazardous Materials, 447, 130773. https://doi.org/10.1016/J.JHAZMAT.2023.130773 DOI: https://doi.org/10.1016/j.jhazmat.2023.130773
Liu, C., Lin, J., Cao, H., Zhang, Y., & Sun, Z. (2019). Recycling of spent lithium-ion batteries in view of lithium recovery: A critical review. Journal of Cleaner Production, 228, 801-813. https://doi.org/10.1016/J.JCLEPRO.2019.04.304 DOI: https://doi.org/10.1016/j.jclepro.2019.04.304
Lv, H., Huang, H., Huang, C., Gao, Q., Yang, Z., & Zhang, W. (2021). Electric field driven de-lithiation: A strategy towards comprehensive and efficient recycling of electrode materials from spent lithium ion batteries. Applied Catalysis B: Environmental, 283, 119634. https://doi.org/10.1016/J.APCATB.2020.119634 DOI: https://doi.org/10.1016/j.apcatb.2020.119634
Magdalon, I. M. (2021). Valorização das Baterias de Iões Lítio em Fim de Vida de Veículos Elétricos. Instituto Politecnico de Leiria.
Makuza, B., Tian, Q., Guo, X., Chattopadhyay, K., & Yu, D. (2021). Pyrometallurgical options for recycling spent lithium-ion batteries: A comprehensive review. Journal of Power Sources, 491, 229622. https://doi.org/10.1016/J.JPOWSOUR.2021.229622 DOI: https://doi.org/10.1016/j.jpowsour.2021.229622
Mantuano, D. P., Espinosa, D. C. R., Wolff, E., Mansur, M. B., & Schwabe, W. K. (2011). Pilhas e baterias portáteis: legislação, processos de reciclagem e perspectivas. Brazilian Journal of Environmental Sciences (RBCIAMB), 21, 1–13.
Mishra, G., Jha, R., Meshram, A., & Singh, K. K. (2022). A review on recycling of lithium-ion batteries to recover critical metals. Journal of Environmental Chemical Engineering, 10(6), 108534. https://doi.org/10.1016/J.JECE.2022.108534 DOI: https://doi.org/10.1016/j.jece.2022.108534
Moazzam, P., Boroumand, Y., Rabiei, P., Baghbaderani, S. S., Mokarian, P., Mohagheghian, F., Mohammed, L. J., & Razmjou, A. (2021). Lithium bioleaching: An emerging approach for the recovery of Li from spent lithium ion batteries. Chemosphere, 277, 130196. https://doi.org/10.1016/J.CHEMOSPHERE.2021.130196 DOI: https://doi.org/10.1016/j.chemosphere.2021.130196
Mossali, E., Picone, N., Gentilini, L., Rodrìguez, O., Pérez, J. M., & Colledani, M. (2020). Lithium-ion batteries towards circular economy: A literature review of opportunities and issues of recycling treatments. Journal of Environmental Management, 264, 110500. https://doi.org/10.1016/J.JENVMAN.2020.110500 DOI: https://doi.org/10.1016/j.jenvman.2020.110500
Pang, J., Liu, Z., Hou, W., & Tao, Y. (2023). How does the Paris Agreement affect firm productivity? International evidence. Finance Research Letters, 56, 104150. https://doi.org/10.1016/J.FRL.2023.104150 DOI: https://doi.org/10.1016/j.frl.2023.104150
Pinegar, H., & Smith, Y. R. (2019). Recycling of End-of-Life Lithium Ion Batteries, Part I: Commercial Processes. Journal of Sustainable Metallurgy, 5(3), 402-416. https://doi.org/10.1007/S40831-019-00235-9/FIGURES/8 DOI: https://doi.org/10.1007/s40831-019-00235-9
Rautela, R., Yadav, B. R., & Kumar, S. (2023). A review on technologies for recovery of metals from waste lithium-ion batteries. Journal of Power Sources, 580, 233428. https://doi.org/10.1016/J.JPOWSOUR.2023.233428 DOI: https://doi.org/10.1016/j.jpowsour.2023.233428
Roy, J. J., Cao, B., & Madhavi, S. (2021). A review on the recycling of spent lithium-ion batteries (LIBs) by the bioleaching approach. Chemosphere, 282, 130944. https://doi.org/10.1016/J.CHEMOSPHERE.2021.130944 DOI: https://doi.org/10.1016/j.chemosphere.2021.130944
Roy, J. J., Madhavi, S., & Cao, B. (2021). Metal extraction from spent lithium-ion batteries (LIBs) at high pulp density by environmentally friendly bioleaching process. Journal of Cleaner Production, 280, 124242. https://doi.org/10.1016/J.JCLEPRO.2020.124242 DOI: https://doi.org/10.1016/j.jclepro.2020.124242
S. Rangarajan, S., Sunddararaj, S. P., Sudhakar, A. V. V., Shiva, C. K., Subramaniam, U., Collins, E. R., & Senjyu, T. (2022). Lithium-Ion Batteries—The Crux of Electric Vehicles with Opportunities and Challenges. Clean Technologies, 4(4), 908-930. https://doi.org/10.3390/CLEANTECHNOL4040056 DOI: https://doi.org/10.3390/cleantechnol4040056
Salman, M., Long, X., Wang, G., & Zha, D. (2022). Paris climate agreement and global environmental efficiency: New evidence from fuzzy regression discontinuity design. Energy Policy, 168, 113128. https://doi.org/10.1016/J.ENPOL.2022.113128 DOI: https://doi.org/10.1016/j.enpol.2022.113128
Silva, N. F. S. F., Ferreira, G. K., Reis, E. P., & Castro, D. E. (2019). A importância da reciclagem na sustentabilidade de carros elétricos. Conexão Ciência (Online), 14(3), 9-18. https://doi.org/10.24862/CCO.V14I3.1044 DOI: https://doi.org/10.24862/cco.v14i3.1044
Singh, J. (2022). The Sustainability Potential of Upcycling. Sustainability, 14(10), 5989. https://doi.org/10.3390/SU14105989 DOI: https://doi.org/10.3390/su14105989
UNEP. (2023). Electric Vehicle Lithium-ion Batteries in Lower- and Middle-income Countries . UNEP - UN Environment Programme.
USGS. (2023). Mineral commodity summaries 2023.
Valorcar. (2019). Guia de Gestão de Resíduios de Baterias e Acumuladores.
Velázquez-Martínez, O., Valio, J., Santasalo-Aarnio, A., Reuter, M., & Serna-Guerrero, R. (2019). A Critical Review of Lithium-Ion Battery Recycling Processes from a Circular Economy Perspective. Batteries, 5(4), 68. https://doi.org/10.3390/BATTERIES5040068 DOI: https://doi.org/10.3390/batteries5040068
Wei, G., Liu, Y., Jiao, B., Chang, N., Wu, M., Liu, G., Lin, X., Weng, X. F., Chen, J., Zhang, L., Zhu, C., Wang, G., Xu, P., Di, J., & Li, Q. (2023). Direct recycling of spent Li-ion batteries: Challenges and opportunities toward practical applications. IScience, 26(9), 107676. https://doi.org/10.1016/J.ISCI.2023.107676 DOI: https://doi.org/10.1016/j.isci.2023.107676
Xin, Y., Guo, X., Chen, S., Wang, J., Wu, F., & Xin, B. (2016). Bioleaching of valuable metals Li, Co, Ni and Mn from spent electric vehicle Li-ion batteries for the purpose of recovery. Journal of Cleaner Production, 116, 249-258. https://doi.org/10.1016/J.JCLEPRO.2016.01.001 DOI: https://doi.org/10.1016/j.jclepro.2016.01.001
Yang, K., Zhu, C., Li, J., Meng, B., Zhong, K., Huang, W., Yu, J., & Fang, Z. (2023). Electric field-assisted leaching of valuable metals from spent lithium-ion batteries in a mixture of acetic acid and ascorbic acid. Hydrometallurgy, 221, 106152. https://doi.org/10.1016/J.HYDROMET.2023.106152 DOI: https://doi.org/10.1016/j.hydromet.2023.106152
Yu, W., Guo, Y., Xu, S., Yang, Y., Zhao, Y., & Zhang, J. (2023). Comprehensive recycling of lithium-ion batteries: Fundamentals, pretreatment, and perspectives. Energy Storage Materials, 54, 172-220. https://doi.org/10.1016/J.ENSM.2022.10.033 DOI: https://doi.org/10.1016/j.ensm.2022.10.033
Zhang, G., Yuan, X., Tay, C. Y., He, Y., Wang, H., & Duan, C. (2023). Selective recycling of lithium from spent lithium-ion batteries by carbothermal reduction combined with multistage leaching. Separation and Purification Technology, 314, 123555. https://doi.org/10.1016/J.SEPPUR.2023.123555 DOI: https://doi.org/10.1016/j.seppur.2023.123555
Zhang, N., Xu, Z., Deng, W., & Wang, X. (2022). Recycling and Upcycling Spent LIB Cathodes: A Comprehensive Review. Electrochemical Energy Reviews, 5(1), 1-38. https://doi.org/10.1007/S41918-022-00154-6 DOI: https://doi.org/10.1007/s41918-022-00154-6
Downloads
Published
How to Cite
Issue
Section
License
Copyright (c) 2024 Brazilian Journal of Production Engineering
This work is licensed under a Creative Commons Attribution-NonCommercial-ShareAlike 4.0 International License.